Synthesis and characterization of a structure H hydrate formed with carbon dioxide and 3,3-dimethyl-2-butanone.

نویسندگان

  • Kyoichi Tezuka
  • Renkai Shen
  • Taku Watanabe
  • Satoshi Takeya
  • Saman Alavi
  • John A Ripmeester
  • Ryo Ohmura
چکیده

Experiments were carried out to synthesize and characterize a structure H clathrate hydrate containing CO(2) and 3,3-dimethyl-2-butanone (pinacolone) by means of phase equilibrium and powder X-ray diffraction measurements. Molecular dynamics simulations of this structure H hydrate were performed to understand the nature of guest-host molecular interactions.

برای دانلود رایگان متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Synthesis, Characterization, and Crystal Structure Determination of Iron(III) Hetero-ligand Complex Containing Chloride, Dimethyl sulfoxide, pyridine-2, 6-dicarboxylate and Water, [Fe(Pydc)(DMSO)(H2O)Cl]

A new metal-organic compound, [Fe(Pydc)(DMSO)(H2O)Cl], (where Pydc is pyridine-2, 6-dicarboxylate and DMSO is dimethyl sulfoxide), has been synthesized and characterized by singlecrystal X-ray diffraction, TGA/DTA, IR and Raman spectroscopy. Green-yellow crystals,crystallized in the monoclinic system, space group P21/n, a = 7.2461(4) Å, b = 10.3018(4) Å, c =17.7667(10) Å, α = 90°, β = 90.014°(5...

متن کامل

Synthesis, Characterization and Crystal Structure Determination of Copper (II) Complexes with 2,2′-Dimethyl-4,4′-bithiazole

Copper(II)  complex  [Cu(dmbt)2(H2O)](ClO4)2 (1)  was  prepared  from  the  reaction  of  copper(II) perchlorate  hexahydrate  with  2,2'-dimethyl-4,4'-bithiazole  (dmbt)  ligand  in  methanol  at  ambient temperature. The complex was quantitatively and qualitatively characterized by elemental analysis, absorption  and  infrared  spectrometries.  Complex  [Cu(DMSO)5](ClO4)2 (2)  was  also  synt...

متن کامل

One-dimensional Uranium(VI) Coordination Polymer Complex Containing Dimethyl and Trimethyl Phosphate Ligands: Synthesis, Spectroscopic Characterization, Thermal Analyses, and Crystal Structure

A new one-dimensional uranium(VI) coordination polymer, [UO2(μ-DMP)2(TMP)]n (1) (DMP is dimethyl phosphate and TMP is trimethyl phosphate), was prepared from the reaction of UO2(NO3)2.6H2O and TMP in in THF (THF is tetrahydrofuran) as a solvent. Suitable crystals of this complex for crystal structure determination were obtained by slow evaporation of the produced yellow solution at room tempera...

متن کامل

Synthesis and Characterization of Anatase-coated Multiwall Carbon Nanotube for Improvement of Photocatalytic Activity

Sol-gel technique was used to coat multiwall carbon nanotubes (MWCNTs) with anatase titania to increasing the surface area and improve the photocatalytic activity of TiO2. Room temperature ballistic conduct of MWCNT combined with semiconducting behavior of anatase brought about a photocatalytic improvement of ~37 % with respect to the highest methyl orange decolorization flair. For characteriza...

متن کامل

Synthesis and Characterization of Silver/Alumina Powders

In this research, synthesis and characterization of silver/alumina composite powders was investigated. This kind of metal/ceramic composite powders is used for fabrication of cutting tools inserts. The role of silver is toughening the final product. The powders were synthesized via co-precipitation method. The composition of the synthesized powders was Ag/80% wt 〖Al〗_2 O_3. Silver nitrate, alum...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

عنوان ژورنال:
  • Chemical communications

دوره 49 5  شماره 

صفحات  -

تاریخ انتشار 2013